andem Catalyst and Process for Enhanced Alkane Dehydrogenation Yield

SHORT DESCRIPTION

For chemical processing plants, this catalyst system produces olefins with record per-pass yields by integrating propane dehydrogenation and selective hydrogen combustion in one reactor.

INVENTORS
  • Justin Notestein*
    • Chair and Professor of Chemical and Biological Engineering, Northwestern University McCormick School of Engineering
  • Peter Stair*
    • Professor of Chemistry Emeritus, Northwestern University, Weinberg College of Arts and Sciences
  • Huan Yan

*Principal Investigator

NU Tech ID: 2020-057

IP STATUS

Issued US Patent 12,311,343

DEVELOPMENT STAGE

TRL-4 - Prototype Validated in Lab: A laboratory-scale prototype has demonstrated integration of tandem catalytic functions with significant performance improvements.

 

BACKGROUND

Current dehydrogenation methods use either multiple reactors with complex layouts or catalysts that suffer from poor selectivity due to oxidation. Engineered solutions require expensive re-heaters and staged reactors, while catalytic methods often fail to overcome equilibrium limitations, driving the need for a simplified, efficient approach.

ABSTRACT

The invention integrates a tandem catalyst design using atomic layer deposition to coat a platinum-alumina catalyst with indium oxide in a core-shell configuration. This spatially organized structure protects the propane dehydrogenation catalyst from oxidation while driving selective hydrogen combustion. The process shifts the equilibrium, achieving a record ~40% per-pass yield of propylene. Laboratory tests confirm catalyst stability and consistent selectivity across increased conversions.

MARKET OPPORTUNITY

The global petrochemical market, valued at $623.8 billion in 2023, is under immense pressure to increase efficiency and reduce its significant energy footprint (Source: Fortune Business Insights, 2024). A critical segment within this industry is the refinery catalyst market, which was valued at $4.82 billion in 2023 and is driven by the constant need for process optimization (Source: Fortune Business Insights, 2024).

A primary operational bottleneck is the high cost and inefficiency of current dehydrogenation processes, which rely on complex, multi-reactor layouts with expensive re-heaters to manage high energy demands. Furthermore, conventional catalysts suffer from poor selectivity and deactivation due to coke buildup, leading to costly downtime. This technology directly addresses this multi-billion dollar unmet need by providing a simplified, highly efficient catalytic approach that overcomes equilibrium limitations, reduces capital expenditure, and minimizes energy consumption.

APPLICATIONS

  • Catalysts for alkane dehydrogenation: Ideal for converting propane to propylene and similar transformations.
  • Alcohol dehydrogenation: Applicable for dehydrogenating alcohols to produce aldehydes and ketones.
  • Tandem reaction systems: Coupling dehydrogenation with selective hydrogen combustion to drive equilibrium.
  • Sugars and alcohol coupling reactions: Suitable for processes such as ethanol to ethyl acetate conversion.
ADVANTAGES
  • Increases per-pass yield: Achieves ~40% propylene yield compared to ~30% with incumbent catalysts.
  • Simplifies reactor design: Combines dual reactions in a single reactor, reducing cost and complexity.
  • Enhances catalyst stability: The core-shell structure minimizes sintering and deactivation.
  • Improves selectivity: Operates under oxidizing conditions without compromising PDH catalyst performance.
PUBLICATIONS
Patent Information: